unbind

1. To remove a band from free from fastenings .

2. To set free .

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1. To release from restraints or bonds; free.

2. To untie or unfasten, as wrappings or bindings.

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Here are some other words you could make with the letters unbind, you can also
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Top Words by points	Points	Word Game
unbind	9	Scrabble

2 Letters	Scrabble® Points
bi	4
un	2
nu	2
in	2
id	3

3 Letters	Scrabble® Points
bid	6
uni	3
nun	3
nub	5
nib	5
inn	3
dun	4
dui	4
dub	6
din	4
dib	6
bun	5
bud	6
bin	5

4 Letters	Scrabble® Points
bunn	6
bund	7
bind	7

5 Letters	Scrabble® Points
unbid	8

6 Letters	Scrabble® Points
unbind	9